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Towards magnetic resonance in scanning tunneling microscopy using heterodyne detection

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Book Series: Experimental Condensed Matter Physics / Karlsruher Institut für Technologie, Physikalisches Institut ISSN: 21919925 ISBN: 9783731504108 Year: Volume: 18 Pages: 151 p. DOI: 10.5445/KSP/1000048009 Language: ENGLISH
Publisher: KIT Scientific Publishing
Subject: Physics (General)
Added to DOAB on : 2019-07-30 20:01:59
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The present work introduces a new concept for magnetic resonance measurements in the GHz regime inside a scanning tunneling microscope. It is based on heterodyne detection in a spin-polarized tunneling barrier. The experimental requirements, including a new method to suppress transmission effects, are explained. Measurements on three model systems which were studied to validate the new technique are presented and compared to simulations.

Investigation of Magnetic Adatoms with Scanning Tunneling Techniques

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Book Series: Experimental Condensed Matter Physics / Karlsruher Institut für Technologie, Physikalisches Institut ISSN: 21919925 ISBN: 9783731504351 Year: Volume: 19 Pages: II, 99 p. DOI: 10.5445/KSP/1000049666 Language: ENGLISH
Publisher: KIT Scientific Publishing
Subject: Physics (General)
Added to DOAB on : 2019-07-30 20:02:02
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In this work, magnetic atoms on surfaces are studied with low-temperature scanning tunneling microscopy. Motivated by the idea to use single atoms as magnetic bits, the factors that allow or prevent long-term stability of their magnetic moments are investigated. Lifetimes of up to several minutes can be achieved for the magnetic moments of holmium atoms on a Pt(111) surface, resulting from the combined symmetries of the system. Corresponding theoretical calculations are presented and evaluated.

Polarization Phenomena in Physics:Applications to Nuclear Reactions

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ISBN: 9789813230897 Year: Pages: 156 DOI: 10.1142/10731 Language: English
Publisher: World Scientific Publishing Co.
Added to DOAB on : 2018-05-02 05:44:00
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This book allows the reader to understand the fundamentals of polarization phenomena in a general spin system, showing the polarizations to be indispensable information source of spin-dependent interactions. Particularly, the book describes polarization phenomena in nuclear scattering and reactions in detail, and explains how they provide information concerning spin-dependent interactions between the related particles. The concepts of polarization observables are explained, explicitly in the scattering of protons, deuterons and 7Li nuclei. In looking at deuteron and 7Li scattering, interactions induced by the virtual excitation of projectiles are examined in detail. Resonance reactions are investigated, focusing attention on the polarization of observables, which suggests that polarization phenomena can be used to determine the spin parity of the resonance. It is noted that in few-nucleon systems, the discrepancy between the values of polarization observables based on theoretical models and the corresponding values obtained through experimental data, is an important problem to be solved in the future. Solving this problem should provide new knowledge concerning the nuclear forces between nucleons.The author has chosen open-access publishing for this book to allow any interested person to study this branch of nuclear physics.

Spin-Crossover Complexes

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ISBN: 9783038428251 9783038428268 Year: Pages: VI, 200 Language: English
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: Chemistry (General)
Added to DOAB on : 2018-06-26 14:01:59
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The spin-crossover (SCO) phenomenon originates from the intrinsic bistability of the d-electron configuration, created by the competition between ligand-field splitting and spin-pairing energies in a first coordination sphere of transition metal ions. Since Cambi’s visionary finding of the SCO phenomenon in 1931, considerable knowledge concerning syntheses, crystal structures, magnetic and thermodynamic properties, spectroscopies, molecular orbital calculations, and theories of SCO complexes has accumulated in a very large number of inorganic molecular coordination compounds, and, in addition, inorganic cobaltates and bioinorganic molecular systems. Recent studies which have focused on other electronic properties exhibited by SCO complexes themselves, control of molecular assemblies, and moreover, multifunctionalization of SCO complexes with either different electronic properties or porous frameworks will open the possibility toward future practical applications of SCO complexes. Thus, the fundamentals and applications of SCO complexes afford a very exciting research field in inorganic coordination chemistry and continues to attract growing attention on a wide range of relevant research fields. This Special Issue aims at collecting research and review contributions concerning recent advances in all aspects of SCO and related phenomena and disseminating this extensive knowledge with a broader audience by means of open access publishing. I invite you to contribute papers in the following research areas so that your research can impact the next generation trends in this promising field.

Explizit korrelierte quasirelativistische Wellenfunktionen

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ISBN: 9783866443990 Year: Pages: IV, 78 p. DOI: 10.5445/KSP/1000012165 Language: GERMAN
Publisher: KIT Scientific Publishing
Subject: Chemistry (General)
Added to DOAB on : 2019-07-30 20:02:02
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Die Arbeit befasst sich mit der Kombination von explizit korrelierten Wellenfunktionen mit quasirelativistischen Hamilton-Operatoren. Die relativistische MP2-R12-Methode wurde entwickelt und effizient implementiert, um molekulare Systeme behandeln zu können. Es werden der skalare DKH- und Pauli-Operator, und zweikomponentige Spin-Bahn-ECPs behandelt. Der Basissatzfehler wird durch die R12-Terme drastisch reduziert, relativistische Effekte werden konsistent in die Störentwicklung einbezogen.

Synthesis and Applications of New Spin Crossover Compounds

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ISBN: 9783039213610 9783039213627 Year: Pages: 254 DOI: 10.3390/books978-3-03921-362-7 Language: English
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: Science (General) --- Physics (General)
Added to DOAB on : 2019-12-09 11:49:15
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The crystal chemistry of spin crossover (SCO) behavior in coordination compounds can potentially be in association with smart materials—promising materials for applications as components of memory devices, displays, sensors and mechanical devices and, especially, actuators, such as artificial muscles. This Special Issue is devoted to various aspects of SCO and related research, comprising 18 interesting original papers on valuable and important SCO topics. Significant and fundamental scientific attention has been focused on the SCO phenomena in a wide research range of fields of fundamental chemical and physical and related sciences, containing the interdisciplinary regions of chemical and physical sciences related to the SCO phenomena. Coordination materials with bistable systems between the LS and the HS states are usually triggered by external stimuli, such as temperature, light, pressure, guest molecule inclusion, soft X-ray, and nuclear decay. Since the first Hofmann-like spin crossover (SCO) behavior in {Fe(py)2[Ni(CN)4]}n (py = pyridine) was demonstrated, this crystal chemistry motif has been frequently used to design Fe(II) SCO materials to enable determination of the correlations between structural features and magnetic properties.

Keywords

spin crossover --- spin transition --- cobalt(II) ion --- paramagnetic ligand --- aminoxyl --- switch --- mosaicity --- spin crossover --- X-ray diffraction --- fatigability --- single crystal --- phase transition --- structural disorder --- spin-crossover --- dinuclear triple helicate --- Fe(II) --- solvent effects --- metal dithiolene complexes --- [Au(dmit)2]?, [Au(dddt)2]? --- ion-pair crystals --- [Fe(III)(3-OMesal2-trien)]+ --- coordination complexes --- crystal structure --- magnetic properties --- magnetic susceptibility --- magnetization --- spin-crossover transition --- Fe(II) complex --- dipyridyl-N-alkylamine ligands --- high spin (HS) --- low spin (LS) --- spin cross-over (SCO) --- magnetic transition --- cobalt oxide --- spin polaron --- impurity effect --- spin-state crossover --- coordination polymer --- supramolecular isomerism --- spin crossover --- crystal engineering --- spin crossover --- X-ray absorption spectroscopy --- soft X-ray induced excited spin state trapping --- high spin --- spin-crossover --- LIESST effect --- hydrogen bonding --- ?-? interactions --- charge-transfer phase transition --- iron mixed-valence complex --- hetero metal complex --- dithiooxalato ligand --- substitution of 3d transition metal ion --- ferromagnetism --- dielectric response --- 57Fe Mössbauer spectroscopy --- Fe(III) coordination complexes --- hexadentate ligand --- Schiff base --- spin crossover --- UV-Vis spectroscopy --- SQUID --- EPR spectroscopy --- spin-crossover --- optical microscopy --- reaction diffusion --- spin crossover --- Fe(III) complex --- qsal ligand --- thermal hysteresis --- structure phase transition --- counter-anion --- solvate --- lattice energy --- optical conductivity spectrum --- spiral structure --- 1,2-bis(4-pyridyl)ethane --- supramolecular coordination polymer --- chiral propeller structure --- atropisomerism --- spin crossover --- iron(II) complexes --- C–H···? interactions --- magnetic properties --- thermochromism --- spin crossover --- linear pentadentate ligand --- iron(II) --- mononuclear --- 1,2,3-triazole --- crystal structure --- magnetic properties --- DFT calculation --- intermolecular interactions --- amorphous --- spin crossover --- Cu(II) complexes --- nitroxides --- phase transitions --- magnetostructural correlations --- iron (II), spin crossover --- X-ray diffraction --- coordination polymers --- n/a

Magnetic Resonance Sensors

ISBN: 9783906980980 9783906980997 Year: Pages: 224 Language: English
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Added to DOAB on : 2015-10-22 09:04:48
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Magnetic Resonance finds applications, from spectroscopy to imaging, on a routine basis in the majority of research and medical institutions. It is also becoming more frequently used for specific applications in which the whole instrument and system is designed for optimum operation. Magnetic Resonance sensors have been applied to fields as varied as petro-chemistry - with borehole logging, food engineering - with online process monitoring, emergency medicine - with point of care diagnostics and civil engineering - with sensors for monitoring cement drying. This great diversity is seeing exciting developments in magnetic resonance sensing technology published in application specific journals where they are often not seen by the wider sensor community.

Higher Spin Gauge Theories

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ISBN: 9783038429975 9783038429982 Year: Pages: X, 448 Language: english
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: Physics (General) --- Mathematics
Added to DOAB on : 2018-08-09 15:16:01
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This book collects various original contributions to the subject of higher spin gauge theory, as well as four review papers on the topic. The papers investigate the role of gauge fields with spin higher than two in the framework of classical and quantum field theories, the AdS/CFT correspondence and string theory.

Advances in Organic Conductors and Superconductors

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ISBN: 9783038971801 9783038971818 Year: Pages: 344 DOI: 10.3390/books978-3-03897-181-8 Language: English
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: Chemistry (General)
Added to DOAB on : 2018-10-04 12:13:06
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ca. 200 words; this text will present the book in all promotional forms (e.g. flyers). Please describe the book in straightforward and consumer-friendly terms.Crystalline conductors and superconductors based on organic molecules are a rapidly progressing field of solid-state science, comprising chemists, and experimental and theoretical physicists from all around the world. In focus are solids with electronic properties governed by delocalized π-electrons. Although carbon-based materials of various shades have gained enormous interest in recent years, charge transfer salts are still paradigmatic in this field. Progress in molecular design is achieved via tiny but ingenious modifications, as well as by fundamentally different approaches. The wealth of exciting physical phenomena is unprecedented and could not have been imagined when the field took off almost half a century ago. Organic low-dimensional conductors are prime examples of Luttinger liquids, exhibit a tendency toward Fermi surface instabilities, but can also be tuned across a dimension¬a¬lity-driven phase diagram like no other system. Superconductivity comes at the border to ordered phases in the spin and charge sectors, and, at high fields, the Fulde–Ferrell–Larkin–Ovchinnikov (FFLO) state is well established. The interplay between charge and magnetic order is still under debate, but electronic ferroelectricity is well established. After decades of intense search, the spin liquid state was first discovered in organic conductors when the amount of geometrical frustration and electronic correlations is just right. They drive the metal and superconductor into an insulating Mott state, solely via electron–electron interactions. However, what do we know about the effect of disorder? Can we tune the electronic properties by pressure, by light, or by field? Research is still addressing basic questions, but devices are not out of reach. These are currently open questions, as well as hot and timely topics. The present Special Issue on “Advances in Organic Conductors and Superconductors” provides a status report summarizing the progress achieved in the last five years.

Hybrid quantum system based on rare earth doped crystals

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Book Series: Experimental Condensed Matter Physics / Karlsruher Institut für Technologie, Physikalisches Institut ISSN: 21919925 ISBN: 9783731503453 Year: Volume: 16 Pages: II, 140 S DOI: 10.5445/KSP/1000045903 Language: ENGLISH
Publisher: KIT Scientific Publishing
Subject: Physics (General)
Added to DOAB on : 2019-07-30 20:02:00
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Hybrid quantum circuits interfacing rare earth spin ensembles with microwave resonators are a promising approach for application as coherent quantum memory and frequency converter. In this thesis, hybrid circuits based on Er and Nd ions doped into Y?SiO? and YAlO? crystals are investigated by optical and on-chip microwave spectroscopy. Coherent strong coupling between the microwave resonator and spin ensemble as well as a multimode memory for weak coherent microwave pulses are demonstrated.

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