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Selektive katalysierte Reduktion von NOx mittels NH3 an Fe-modifizierten BEA-Zeolithen

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ISBN: 9783866447066 Year: Pages: 190 p. DOI: 10.5445/KSP/1000023659 Language: GERMAN
Publisher: KIT Scientific Publishing
Subject: Chemistry (General)
Added to DOAB on : 2019-07-30 20:02:00
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In der vorliegenden Arbeit wurde die selektive katalytische Reduktion von NOx mittels Ammoniak an eisenmodifizierten BEA-Zeolithen untersucht. Der Katalysator zeigt gegenüber dem kommerziellen V2O5/WO3/TiO2-System eine bessere tieftemperatur SCR-Aktivität, sowie eine bessere Beständigkeit gegen über hydrothermaler Alterung. Der Prototyp am Motorenprüfstand zeigt eine dem kommerziellen V2O5/TiO2-System identische SCR-Aktivität. Die vorliegenden Eisenspezies werden charakterisiert.

Detaillierte Modellierung der Pt-katalysierten Schadstoffminderung in Abgasen moderner Verbrennungsmotoren

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ISBN: 9783866442931 Year: Pages: XV, 140 p. DOI: 10.5445/KSP/1000009337 Language: GERMAN
Publisher: KIT Scientific Publishing
Subject: Chemistry (General)
Added to DOAB on : 2019-07-30 20:02:02
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Die stetige Verschärfung der Emissionsgrenzwerte von Verbrennungsmotoren seitens des Gesetzgebers erfordert die Weiterentwicklung und Verbesserung von Technologien der katalytischen Abgasnachbehandlung.Das Ziel dieser Arbeit besteht daher in der Weiterentwicklung eines detaillierten, auf Elementarschritten basierenden Reaktionsmechanismus für die Edelmetallkomponente Platin und die Entwicklung eines Modells zur numerischen Simulation eines NOx-Speicher/Reduktionskatalysators (NSC).

Advances in Catalyst Deactivation

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ISBN: 9783038421870 9783038421887 Year: Pages: X, 300 DOI: 10.3390/books978-3-03842-188-7 Language: English
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: Chemical Engineering
Added to DOAB on : 2016-06-07 11:25:06
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Catalyst deactivation, the loss over time of catalytic activity and/or selectivity, is a problem of great and continuing concern in the practice of industrial catalytic processes. Costs to industry for catalyst replacement and process shutdown total tens of billions of dollars per year. While catalyst deactivation is inevitable for most processes, some of its immediate, drastic consequences may be avoided, postponed, or even reversed. Accordingly, there is considerable motivation to better understand catalyst decay and regeneration. Indeed, the science of catalyst deactivation and regeneration has been developing rapidly as evidenced by the considerable literature addressing this topic, including 21,000 journal articles, presentations, reports, reviews, and books; and more than 29,000 patents for the period of 1980 to 2012. This developing science provides the foundation for continuing, substantial improvements in the efficiency and economics of catalytic processes through development of catalyst deactivation models, more stable catalysts, and regeneration processes.This special issue focuses on recent advances in catalyst deactivation and regeneration, including advances in (1) scientific understanding of mechanisms; (2) development of improved methods and tools for investigation; and (3) more robust models of deactivation and regeneration.

Application of Photoactive Nanomaterials in Degradation of Pollutants

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ISBN: 9783039213818 / 9783039213825 Year: Pages: 134 DOI: 10.3390/books978-3-03921-382-5 Language: eng
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: Science (General) --- Chemistry (General)
Added to DOAB on : 2019-12-09 11:49:15
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Photoactive nanomaterials have been receiving increasing attention due to their potential application in the light-driven degradation of water and gas-phase pollutants. However, to exploit the great potential of photoactive materials and access their properties requires fine-tuning of their size/shape-dependent chemical–physical properties, and on the ability to integrate them in photoreactors or to deposit them onto large surfaces. Therefore, the synthetic approach as well as post-synthesis manipulation could strongly affect the final photocatalytic properties of the nanomaterial. The aim of the present Special Issue is to report on the most recent progress towards the application of photoactive nanomaterials and nanomaterial-based coatings in pollutant degradation, paying particular attention to cases close to real application: scalable synthetic approaches to nanocatalysts, preparation of nanocatalyst-based coatings, degradation of real pollutants and bacterial inactivation, and application in building materials.

Plasma Processes for Renewable Energy Technologies

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ISBN: 9783039219728 / 9783039219735 Year: Pages: 118 DOI: 10.3390/books978-3-03921-973-5 Language: eng
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: General and Civil Engineering --- Technology (General)
Added to DOAB on : 2020-01-30 16:39:46
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The use of renewable energy is an effective solution for the prevention of global warming. On the other hand, environmental plasmas are one of powerful means to solve global environmental problems on nitrogen oxides, (NOx), sulfur oxides (SOx), particulate matter (PM), volatile organic compounds (VOC), and carbon dioxides (CO2) in the atmosphere. By combining both technologies, we can develop an extremely effective environmental improvement technology. Based on this background, a Special Issue of the journal Energies on plasma processes for renewable energy technologies is planned. On the issue, we focus on environment plasma technologies that can effectively utilize renewable electric energy sources, such as photovoltaic power generation, biofuel power generation, wind turbine power generation, etc. However, any latest research results on plasma environmental improvement processes are welcome for submission. We are looking, among others, for papers on the following technical subjects in which either plasma can use renewable energy sources or can be used for renewable energy technologies: Plasma decomposition technology of harmful gases, such as the plasma denitrification method; Plasma removal technology of harmful particles, such as electrostatic precipitation; Plasma decomposition technology of harmful substances in liquid, such as gas–liquid interfacial plasma; Plasma-enhanced flow induction and heat transfer enhancement technologies, such as ionic wind device and plasma actuator; Plasma-enhanced combustion and fuel reforming; Other environment plasma technologies.

Applications of Computational Intelligence to Power Systems

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ISBN: 9783039217601 / 9783039217618 Year: Pages: 116 DOI: 10.3390/books978-3-03921-761-8 Language: eng
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: Technology (General) --- General and Civil Engineering
Added to DOAB on : 2019-11-08 11:31:56
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Electric power systems around the world are changing in terms of structure, operation, management and ownership due to technical, financial, and ideological reasons. Power systems keep on expanding in terms of geographical areas, asset additions, and the penetration of new technologies in generation, transmission, and distribution. The conventional methods for solving the power system design, planning, operation, and control problems have been extensively used for different applications, but these methods suffer from several difficulties, thus providing suboptimal solutions. Computationally intelligent methods can offer better solutions for several conditions and are being widely applied in electrical engineering applications. This Special Issue represents a thorough treatment of computational intelligence from an electrical power system engineer’s perspective. Thorough, well-organised, and up-to-date, it examines in detail some of the important aspects of this very exciting and rapidly emerging technology, including machine learning, particle swarm optimization, genetic algorithms, and deep learning systems. Written in a concise and flowing manner by experts in the area of electrical power systems who have experience in the application of computational intelligence for solving many complex and difficult power system problems, this Special Issue is ideal for professional engineers and postgraduate students entering this exciting field.

Plasma Catalysis

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ISBN: 9783038977506 Year: Pages: 246 DOI: 10.3390/books978-3-03897-751-3 Language: eng
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: Chemical Engineering --- Technology (General)
Added to DOAB on : 2019-04-05 10:34:31
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Plasma catalysis is gaining increasing interest for various gas conversion applications, such as CO2 conversion into value-added chemicals and fuels, N2 fixation for the synthesis of NH3 or NOx, methane conversion into higher hydrocarbons or oxygenates. It is also widely used for air pollution control (e.g., VOC

Catalysts Deactivation, Poisoning and Regeneration

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ISBN: 9783039215461 / 9783039215478 Year: Pages: 254 DOI: 10.3390/books978-3-03921-547-8 Language: eng
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: Technology (General) --- Chemical Engineering
Added to DOAB on : 2019-12-09 11:49:15
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Catalyst lifetime represents one of the most crucial economic aspects in industrial catalytic processes, due to costly shutdowns, catalyst replacements, and proper disposal of spent materials. Not surprisingly, there is considerable motivation to understand and treat catalyst deactivation, poisoning, and regeneration, which causes this research topic to continue to grow. The complexity of catalyst poisoning obviously increases along with the increasing use of biomass/waste-derived/residual feedstocks and with requirements for cleaner and novel sustainable processes. This book collects 15 research papers providing insights into several scientific and technical aspects of catalyst poisoning and deactivation, proposing more tolerant catalyst formulations, and exploring possible regeneration strategies.

Keywords

hydrogenation --- copper --- catalyst --- water --- deactivation --- octanal --- octanol --- V2O5–WO3/TiO2 catalysts --- poisoning --- sulfur-containing sodium salts --- SO3 --- NO removal --- Cu/SSZ-13 --- NH3-SCR --- sodium ions --- deactivation mechanism --- sulfur poisoning --- coke deposition --- in situ regeneration --- Co-Zn/H-Beta --- NOx reduction by C3H8 --- catalyst deactivation --- diesel --- natural gas --- SEM --- TEM --- poisoning --- oxygen storage capacity --- thermal stability --- cyclic operation --- deactivation --- oxysulfate --- oxysulfide --- Selective Catalytic Reduction (SCR) --- SO2 poisoning --- Low-temperature catalyst --- nitrogen oxides --- nitrous oxide --- dry reforming of methane --- nickel catalysts --- barium carbonate --- deactivation by coking --- catalytic methane combustion --- exhaust gas --- catalyst durability --- Liquefied natural gas --- biogas --- vehicle emission control --- sulfur deactivation --- catalyst deactivation --- aluminum sulfate --- palladium sulfate --- regeneration --- phthalic anhydride --- vanadia-titania catalyst --- unusual deactivation --- physico-chemical characterization --- over-reduction --- vanadia species --- coke deposition --- DeNOx --- MW incinerator --- deactivation --- ammonium sulfates --- regeneration --- washing --- CO2 reforming --- Ni-catalyst --- syngas --- tetragonal zirconia --- phase stabilization --- CPO reactor --- effect of flow rate --- deactivation --- iso-octane --- Rh catalysts --- Rh --- homogeneous catalysis --- catalyst deactivation --- n/a

Biomass Chars: Elaboration, Characterization and Applications ?

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ISBN: 9783039216628 / 9783039216635 Year: Pages: 342 DOI: 10.3390/books978-3-03921-663-5 Language: eng
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: Agriculture (General) --- Biology --- Science (General)
Added to DOAB on : 2019-12-09 11:49:15
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Biomass can be converted to energy, biofuels, and bioproducts via thermochemical conversion processes, such as combustion, pyrolysis, and gasification. Combustion technology is most widely applied on an industrial scale. However, biomass gasification and pyrolysis processes are still in the research and development stage. The major products from these processes are syngas, bio-oil, and char (called also biochar for agronomic application). Among these products, biomass chars have received increasing attention for different applications, such as gasification, co-combustion, catalysts or adsorbents precursors, soil amendment, carbon fuel cells, and supercapacitors. This Special Issue provides an overview of biomass char production methods (pyrolysis, hydrothermal carbonization, etc.), characterization techniques (e.g., scanning electronic microscopy, X-ray fluorescence, nitrogen adsorption, Raman spectroscopy, nuclear magnetic resonance spectroscopy, X-ray photoelectron spectroscopy, and temperature programmed desorption and mass spectrometry), their properties, and their suitable recovery processes.

Keywords

biomass production --- multicriteria model --- ELECTRE III --- combustion --- oxygen enrichment --- low-rank coal char --- char oxidation --- reaction kinetics --- salty food waste --- FT-IR --- pyrolysis --- biochar --- NaCl --- hydrothermal carbonization --- anaerobic digestion --- poultry slaughterhouse --- sludge cake --- energy recovery efficiency --- gasification --- kinetic model --- active site --- chemisorption --- hydrothermal carbonization (HTC) --- Chinese reed --- biocrude --- biochar --- high heating value (HHV) --- biochar --- steam --- gasification --- chemical speciation --- AAEMs --- underground coal gasification --- ash layer --- effective diffusion coefficient --- internal diffusion resistance --- pyrolysis --- hydrothermal carbonization --- biochar engineering --- porosity --- nutrients --- polycyclic aromatic hydrocarbon (PAH) --- nitrogen --- biomass --- amino acid --- pyrrole --- NOx --- pyrolysis --- grape marc --- kinetic models --- characterization --- pyrolysis --- Texaco pilot plant --- reactor modelling --- ash fusion temperature (AFT) --- melting phenomenon --- food waste compost --- sawdust --- pyrolysis --- biochar --- thermogravimetric analysis (TGA) --- calorific value --- biogas purification --- coconut shells --- biomass valorization --- textural characterization --- adsorption isotherms --- breakthrough curves --- olive mill solid wastes (OMSWs) --- fixed bed combustor --- pellets --- combustion parameters --- gaseous emissions --- waste wood --- interactions --- interferences --- partial combustion reaction in gasification --- Boudouard reaction in gasification --- MTDATA --- biomass --- steam gasification --- kinetics --- pyrolysis conditions --- thermogravimetric analysis --- characteristic time analysis --- biomass --- combustion --- thermogravimetric analysis --- kinetic parameters --- thermal characteristics --- food waste --- food-waste biochar --- pyrolysis --- NaCl template --- desalination --- biochar --- ash from biomass --- giant miscanthus --- fertilisation --- CO2 adsorption --- CH4 adsorption --- biomass --- activated carbon --- n/a

Carbon Based Electronic Devices

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ISBN: 9783039282326 / 9783039282333 Year: Pages: 258 DOI: 10.3390/books978-3-03928-233-3 Language: eng
Publisher: MDPI - Multidisciplinary Digital Publishing Institute
Subject: General and Civil Engineering --- Technology (General)
Added to DOAB on : 2020-04-07 23:07:08
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For more than 50 years, silicon has dominated the electronics industry. However, this growth will come to an end, due to resources limitations. Thus, research developments need to focus to alternative materials, with higher performance and better functionality. Current research achievements have indicated that carbon is one of the promising candidates for its exploitation in the electronics industry. Whereas the physical properties of graphite and diamond have been investigated for many years, the potential for electronic applications of other allotropes of carbon (fullerenes, carbon nanotubes, carbon nanofibres, carbon films, carbon balls and beads, carbon fibers, etc), has only been appreciated relatively recently. Carbon-based materials offer a number of exciting possibilities for new applications of electronic devices, due to their unique thermal and electrical properties. However, the success of carbon-based electronics depends on the rapid progress of the fabrication, doping and manipulation techniques. In this Special Issue, we focus on both insights and advancements in carbon-based electronics. We will also cover various topics ranging from synthesis, functionalisation, and characterisation of carbon-based materials, for their use in electronic devices, including advanced manufacturing techniques, such as 3D printing, ink-jet printing, spray-gun technique, etc.

Keywords

ionization sensor array --- NOx --- carbon nanotube (CNT) --- selectivity --- non-self-sustaining discharge --- carbon nanotube --- field emitters --- electrical aging --- Joule heating --- electron emission --- photosensor --- reduced graphene oxide --- Ag nanoparticles --- solution process --- finite-difference time-domain --- carbon nanofibres (CNFs) --- active-screen plasma sputtering (ASPS) technology --- supercapacitors (SCs) --- silver (Ag) --- platinum (Pt) and palladium (Pd) nanoparticles --- transparent conducting electrode --- flexible electrode --- graphene --- optoelectronic device --- graphene --- Galinstan --- Liquid-Metal --- spray-on --- aerosol --- honey --- mobility --- contact resistance --- TLM --- I-V characteristics --- porous electrode --- pressure sensitivity --- self-powered sensors --- mechanical impact --- carbon nanofillers --- electrical conductivity --- piezoresistive behavior --- ReRAM --- carbon nanofibers --- spray-gun deposition --- carbon Inks --- rheology --- additive manufacturing --- graphene --- carbon nanotubes --- printing --- supercapacitors --- graphene oxide --- metal nanoparticles --- dodecylbenzene sulfonic acid (DBSA) doped polyaniline --- capacitance --- humidity sensor --- carbon-based materials --- carbon nanotubes --- graphene --- carbon black --- carbon fibers --- carbon soot --- biochar --- flexible electronics --- carbon nanotubes --- graphene --- carbon fibres --- functionalization --- supercapacitors --- sensors --- inkjet printer inks --- flexible wearable devices --- electronics --- carbon-based material --- carbon structure differentiation --- NEMS quality --- higher performances --- revised Raman characterization --- quantum electronic activation --- carbon phase transition --- n/a

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